id	sid	tid	token	lemma	pos
70795714n3s	1	1	in	in	ADP
70795714n3s	1	2	this	this	DET
70795714n3s	1	3	dissertation	dissertation	NOUN
70795714n3s	1	4	i	i	PRON
70795714n3s	1	5	present	present	VERB
70795714n3s	1	6	work	work	NOUN
70795714n3s	1	7	on	on	ADP
70795714n3s	1	8	the	the	DET
70795714n3s	1	9	modeling	modeling	NOUN
70795714n3s	1	10	of	of	ADP
70795714n3s	1	11	adsorbate	adsorbate	ADJ
70795714n3s	1	12	-	-	PUNCT
70795714n3s	1	13	metal	metal	NOUN
70795714n3s	1	14	interactions	interaction	NOUN
70795714n3s	1	15	with	with	ADP
70795714n3s	1	16	a	a	DET
70795714n3s	1	17	specific	specific	ADJ
70795714n3s	1	18	focus	focus	NOUN
70795714n3s	1	19	on	on	ADP
70795714n3s	1	20	carbon	carbon	NOUN
70795714n3s	1	21	monoxide	monoxide	NOUN
70795714n3s	1	22	(	(	PUNCT
70795714n3s	1	23	co	co	NOUN
70795714n3s	1	24	)	)	PUNCT
70795714n3s	1	25	induced	induce	VERB
70795714n3s	1	26	restructuring	restructuring	NOUN
70795714n3s	1	27	of	of	ADP
70795714n3s	1	28	platinum	platinum	NOUN
70795714n3s	1	29	stepped	step	VERB
70795714n3s	1	30	surfaces	surface	NOUN
70795714n3s	1	31	.	.	PUNCT
70795714n3s	2	1	additionally	additionally	ADV
70795714n3s	2	2	,	,	PUNCT
70795714n3s	2	3	i	i	PRON
70795714n3s	2	4	will	will	AUX
70795714n3s	2	5	present	present	VERB
70795714n3s	2	6	work	work	NOUN
70795714n3s	2	7	on	on	ADP
70795714n3s	2	8	the	the	DET
70795714n3s	2	9	development	development	NOUN
70795714n3s	2	10	of	of	ADP
70795714n3s	2	11	a	a	DET
70795714n3s	2	12	multiple	multiple	ADJ
70795714n3s	2	13	-	-	PUNCT
70795714n3s	2	14	minima	minima	ADJ
70795714n3s	2	15	fluctuating	fluctuating	NOUN
70795714n3s	2	16	charge	charge	NOUN
70795714n3s	2	17	(	(	PUNCT
70795714n3s	2	18	mm	mm	NOUN
70795714n3s	2	19	-	-	PUNCT
70795714n3s	2	20	flucq	flucq	NOUN
70795714n3s	2	21	)	)	PUNCT
70795714n3s	2	22	potential	potential	NOUN
70795714n3s	2	23	which	which	PRON
70795714n3s	2	24	has	have	AUX
70795714n3s	2	25	been	be	AUX
70795714n3s	2	26	used	use	VERB
70795714n3s	2	27	to	to	PART
70795714n3s	2	28	simulate	simulate	VERB
70795714n3s	2	29	charge	charge	NOUN
70795714n3s	2	30	responsive	responsive	ADJ
70795714n3s	2	31	platinum	platinum	NOUN
70795714n3s	2	32	surfaces.new	surfaces.new	PROPN
70795714n3s	2	33	pt	pt	PROPN
70795714n3s	2	34	-	-	PUNCT
70795714n3s	2	35	co	co	PROPN
70795714n3s	2	36	and	and	CCONJ
70795714n3s	2	37	au	au	PROPN
70795714n3s	2	38	-	-	PUNCT
70795714n3s	2	39	co	co	NOUN
70795714n3s	2	40	forcefields	forcefield	NOUN
70795714n3s	2	41	were	be	AUX
70795714n3s	2	42	developed	develop	VERB
70795714n3s	2	43	to	to	PART
70795714n3s	2	44	study	study	VERB
70795714n3s	2	45	coverage	coverage	NOUN
70795714n3s	2	46	-	-	PUNCT
70795714n3s	2	47	dependent	dependent	ADJ
70795714n3s	2	48	restructuring	restructuring	NOUN
70795714n3s	2	49	of	of	ADP
70795714n3s	2	50	high	high	ADJ
70795714n3s	2	51	-	-	PUNCT
70795714n3s	2	52	index	index	NOUN
70795714n3s	2	53	platinum	platinum	NOUN
70795714n3s	2	54	&	&	CCONJ
70795714n3s	2	55	amp	amp	PROPN
70795714n3s	2	56	;	;	PUNCT
70795714n3s	2	57	gold	gold	NOUN
70795714n3s	2	58	(	(	PUNCT
70795714n3s	2	59	557	557	NUM
70795714n3s	2	60	)	)	PUNCT
70795714n3s	2	61	surfaces	surface	NOUN
70795714n3s	2	62	.	.	PUNCT
70795714n3s	3	1	it	it	PRON
70795714n3s	3	2	was	be	AUX
70795714n3s	3	3	observed	observe	VERB
70795714n3s	3	4	that	that	SCONJ
70795714n3s	3	5	the	the	DET
70795714n3s	3	6	weak	weak	ADJ
70795714n3s	3	7	au	au	X
70795714n3s	3	8	-	-	PUNCT
70795714n3s	3	9	co	co	NOUN
70795714n3s	3	10	binding	binding	NOUN
70795714n3s	3	11	led	lead	VERB
70795714n3s	3	12	to	to	ADP
70795714n3s	3	13	minimal	minimal	ADJ
70795714n3s	3	14	disruption	disruption	NOUN
70795714n3s	3	15	of	of	ADP
70795714n3s	3	16	the	the	DET
70795714n3s	3	17	surface	surface	NOUN
70795714n3s	3	18	,	,	PUNCT
70795714n3s	3	19	whereas	whereas	SCONJ
70795714n3s	3	20	the	the	DET
70795714n3s	3	21	strong	strong	ADJ
70795714n3s	3	22	pt	pt	PROPN
70795714n3s	3	23	-	-	PUNCT
70795714n3s	3	24	co	co	NOUN
70795714n3s	3	25	interactions	interaction	NOUN
70795714n3s	3	26	resulted	result	VERB
70795714n3s	3	27	in	in	ADP
70795714n3s	3	28	significant	significant	ADJ
70795714n3s	3	29	disruption	disruption	NOUN
70795714n3s	3	30	of	of	ADP
70795714n3s	3	31	the	the	DET
70795714n3s	3	32	step	step	NOUN
70795714n3s	3	33	-	-	PUNCT
70795714n3s	3	34	edges	edge	NOUN
70795714n3s	3	35	which	which	PRON
70795714n3s	3	36	led	lead	VERB
70795714n3s	3	37	to	to	ADP
70795714n3s	3	38	increased	increase	VERB
70795714n3s	3	39	step	step	NOUN
70795714n3s	3	40	-	-	PUNCT
70795714n3s	3	41	wandering	wandering	NOUN
70795714n3s	3	42	.	.	PUNCT
70795714n3s	4	1	specifically	specifically	ADV
70795714n3s	4	2	,	,	PUNCT
70795714n3s	4	3	the	the	DET
70795714n3s	4	4	strong	strong	ADJ
70795714n3s	4	5	co	co	NOUN
70795714n3s	4	6	-	-	ADJ
70795714n3s	4	7	co	co	ADJ
70795714n3s	4	8	quadrupolar	quadrupolar	ADJ
70795714n3s	4	9	repulsion	repulsion	NOUN
70795714n3s	4	10	caused	cause	VERB
70795714n3s	4	11	an	an	DET
70795714n3s	4	12	increase	increase	NOUN
70795714n3s	4	13	in	in	ADP
70795714n3s	4	14	adatom	adatom	ADJ
70795714n3s	4	15	mobility	mobility	NOUN
70795714n3s	4	16	.	.	PUNCT
70795714n3s	5	1	this	this	DET
70795714n3s	5	2	increased	increase	VERB
70795714n3s	5	3	mobility	mobility	NOUN
70795714n3s	5	4	eventually	eventually	ADV
70795714n3s	5	5	led	lead	VERB
70795714n3s	5	6	to	to	ADP
70795714n3s	5	7	large	large	ADJ
70795714n3s	5	8	-	-	PUNCT
70795714n3s	5	9	scale	scale	NOUN
70795714n3s	5	10	surface	surface	NOUN
70795714n3s	5	11	reconstructions	reconstruction	NOUN
70795714n3s	5	12	including	include	VERB
70795714n3s	5	13	the	the	DET
70795714n3s	5	14	formation	formation	NOUN
70795714n3s	5	15	of	of	ADP
70795714n3s	5	16	a	a	DET
70795714n3s	5	17	metastable	metastable	ADJ
70795714n3s	5	18	double	double	ADJ
70795714n3s	5	19	layer.a	layer.a	NOUN
70795714n3s	5	20	platinum	platinum	NOUN
70795714n3s	5	21	/	/	SYM
70795714n3s	5	22	palladium	palladium	NOUN
70795714n3s	5	23	(	(	PUNCT
70795714n3s	5	24	pt	pt	PROPN
70795714n3s	5	25	/	/	SYM
70795714n3s	5	26	pd	pd	PROPN
70795714n3s	5	27	)	)	PUNCT
70795714n3s	5	28	(	(	PUNCT
70795714n3s	5	29	557	557	NUM
70795714n3s	5	30	)	)	PUNCT
70795714n3s	5	31	surface	surface	NOUN
70795714n3s	5	32	was	be	AUX
70795714n3s	5	33	simulated	simulate	VERB
70795714n3s	5	34	to	to	PART
70795714n3s	5	35	explore	explore	VERB
70795714n3s	5	36	co	co	ADJ
70795714n3s	5	37	-	-	ADJ
70795714n3s	5	38	induced	induced	ADJ
70795714n3s	5	39	reconstructions	reconstruction	NOUN
70795714n3s	5	40	on	on	ADP
70795714n3s	5	41	a	a	DET
70795714n3s	5	42	more	more	ADV
70795714n3s	5	43	complicated	complicated	ADJ
70795714n3s	5	44	bimetallic	bimetallic	ADJ
70795714n3s	5	45	surface	surface	NOUN
70795714n3s	5	46	.	.	PUNCT
70795714n3s	6	1	the	the	DET
70795714n3s	6	2	pt	pt	PROPN
70795714n3s	6	3	-	-	PUNCT
70795714n3s	6	4	co	co	PROPN
70795714n3s	6	5	forcefield	forcefield	NOUN
70795714n3s	6	6	was	be	AUX
70795714n3s	6	7	retuned	retune	VERB
70795714n3s	6	8	while	while	SCONJ
70795714n3s	6	9	a	a	DET
70795714n3s	6	10	new	new	ADJ
70795714n3s	6	11	pd	pd	PROPN
70795714n3s	6	12	-	-	PUNCT
70795714n3s	6	13	co	co	PROPN
70795714n3s	6	14	forcefield	forcefield	NOUN
70795714n3s	6	15	was	be	AUX
70795714n3s	6	16	developed	develop	VERB
70795714n3s	6	17	.	.	PUNCT
70795714n3s	7	1	the	the	DET
70795714n3s	7	2	difference	difference	NOUN
70795714n3s	7	3	in	in	ADP
70795714n3s	7	4	binding	bind	VERB
70795714n3s	7	5	strengths	strength	NOUN
70795714n3s	7	6	was	be	AUX
70795714n3s	7	7	found	find	VERB
70795714n3s	7	8	to	to	PART
70795714n3s	7	9	play	play	VERB
70795714n3s	7	10	an	an	DET
70795714n3s	7	11	important	important	ADJ
70795714n3s	7	12	role	role	NOUN
70795714n3s	7	13	in	in	ADP
70795714n3s	7	14	the	the	DET
70795714n3s	7	15	disruption	disruption	NOUN
70795714n3s	7	16	of	of	ADP
70795714n3s	7	17	the	the	DET
70795714n3s	7	18	pt	pt	PROPN
70795714n3s	7	19	/	/	SYM
70795714n3s	7	20	pd	pd	PROPN
70795714n3s	7	21	surface	surface	NOUN
70795714n3s	7	22	while	while	SCONJ
70795714n3s	7	23	the	the	DET
70795714n3s	7	24	preferred	preferred	ADJ
70795714n3s	7	25	binding	bind	VERB
70795714n3s	7	26	sites	site	NOUN
70795714n3s	7	27	on	on	ADP
70795714n3s	7	28	each	each	DET
70795714n3s	7	29	system	system	NOUN
70795714n3s	7	30	(	(	PUNCT
70795714n3s	7	31	pt	pt	PROPN
70795714n3s	7	32	:	:	PUNCT
70795714n3s	7	33	atop	atop	PROPN
70795714n3s	7	34	,	,	PUNCT
70795714n3s	7	35	pd	pd	PROPN
70795714n3s	7	36	:	:	PUNCT
70795714n3s	7	37	bridge	bridge	PROPN
70795714n3s	7	38	/	/	SYM
70795714n3s	7	39	hollow	hollow	NOUN
70795714n3s	7	40	)	)	PUNCT
70795714n3s	7	41	led	lead	VERB
70795714n3s	7	42	to	to	ADP
70795714n3s	7	43	significantly	significantly	ADV
70795714n3s	7	44	different	different	ADJ
70795714n3s	7	45	behaviors	behavior	NOUN
70795714n3s	7	46	with	with	ADP
70795714n3s	7	47	regards	regard	NOUN
70795714n3s	7	48	to	to	ADP
70795714n3s	7	49	surface	surface	NOUN
70795714n3s	7	50	diffusion	diffusion	NOUN
70795714n3s	7	51	and	and	CCONJ
70795714n3s	7	52	mobility.the	mobility.the	DET
70795714n3s	7	53	importance	importance	NOUN
70795714n3s	7	54	of	of	ADP
70795714n3s	7	55	step	step	NOUN
70795714n3s	7	56	-	-	PUNCT
70795714n3s	7	57	edge	edge	NOUN
70795714n3s	7	58	energetics	energetic	NOUN
70795714n3s	7	59	for	for	ADP
70795714n3s	7	60	the	the	DET
70795714n3s	7	61	formation	formation	NOUN
70795714n3s	7	62	of	of	ADP
70795714n3s	7	63	adatoms	adatom	NOUN
70795714n3s	7	64	encouraged	encourage	VERB
70795714n3s	7	65	us	we	PRON
70795714n3s	7	66	to	to	PART
70795714n3s	7	67	directly	directly	ADV
70795714n3s	7	68	examine	examine	VERB
70795714n3s	7	69	straight	straight	ADV
70795714n3s	7	70	edged	edge	VERB
70795714n3s	7	71	(	(	PUNCT
70795714n3s	7	72	557	557	NUM
70795714n3s	7	73	)	)	PUNCT
70795714n3s	7	74	&	&	CCONJ
70795714n3s	7	75	amp	amp	PROPN
70795714n3s	7	76	;	;	PUNCT
70795714n3s	7	77	(	(	PUNCT
70795714n3s	7	78	112	112	NUM
70795714n3s	7	79	)	)	PUNCT
70795714n3s	7	80	and	and	CCONJ
70795714n3s	7	81	kinked	kink	VERB
70795714n3s	7	82	edged	edge	VERB
70795714n3s	7	83	(	(	PUNCT
70795714n3s	7	84	765	765	NUM
70795714n3s	7	85	)	)	PUNCT
70795714n3s	7	86	&	&	CCONJ
70795714n3s	7	87	amp	amp	PROPN
70795714n3s	7	88	;	;	PUNCT
70795714n3s	7	89	(	(	PUNCT
70795714n3s	7	90	321	321	NUM
70795714n3s	7	91	)	)	PUNCT
70795714n3s	7	92	platinum	platinum	NOUN
70795714n3s	7	93	surfaces	surface	NOUN
70795714n3s	7	94	.	.	PUNCT
70795714n3s	8	1	as	as	SCONJ
70795714n3s	8	2	expected	expect	VERB
70795714n3s	8	3	,	,	PUNCT
70795714n3s	8	4	the	the	DET
70795714n3s	8	5	systems	system	NOUN
70795714n3s	8	6	with	with	ADP
70795714n3s	8	7	rougher	rougher	ADJ
70795714n3s	8	8	edges	edge	NOUN
70795714n3s	8	9	experienced	experience	VERB
70795714n3s	8	10	a	a	DET
70795714n3s	8	11	greater	great	ADJ
70795714n3s	8	12	amount	amount	NOUN
70795714n3s	8	13	of	of	ADP
70795714n3s	8	14	surface	surface	NOUN
70795714n3s	8	15	diffusion	diffusion	NOUN
70795714n3s	8	16	and	and	CCONJ
70795714n3s	8	17	a	a	DET
70795714n3s	8	18	concomitantly	concomitantly	ADV
70795714n3s	8	19	increased	increase	VERB
70795714n3s	8	20	amount	amount	NOUN
70795714n3s	8	21	of	of	ADP
70795714n3s	8	22	step	step	NOUN
70795714n3s	8	23	-	-	PUNCT
70795714n3s	8	24	wandering	wandering	NOUN
70795714n3s	8	25	.	.	PUNCT
70795714n3s	9	1	the	the	DET
70795714n3s	9	2	length	length	NOUN
70795714n3s	9	3	of	of	ADP
70795714n3s	9	4	the	the	DET
70795714n3s	9	5	(	(	PUNCT
70795714n3s	9	6	111	111	NUM
70795714n3s	9	7	)	)	PUNCT
70795714n3s	9	8	plateaus	plateaus	NOUN
70795714n3s	9	9	between	between	ADP
70795714n3s	9	10	step	step	NOUN
70795714n3s	9	11	edges	edge	NOUN
70795714n3s	9	12	also	also	ADV
70795714n3s	9	13	played	play	VERB
70795714n3s	9	14	an	an	DET
70795714n3s	9	15	important	important	ADJ
70795714n3s	9	16	role	role	NOUN
70795714n3s	9	17	with	with	ADP
70795714n3s	9	18	regard	regard	NOUN
70795714n3s	9	19	to	to	ADP
70795714n3s	9	20	the	the	DET
70795714n3s	9	21	extent	extent	NOUN
70795714n3s	9	22	of	of	ADP
70795714n3s	9	23	surface	surface	NOUN
70795714n3s	9	24	reconstruction	reconstruction	NOUN
70795714n3s	9	25	observed.accurate	observed.accurate	NOUN
70795714n3s	9	26	treatment	treatment	NOUN
70795714n3s	9	27	of	of	ADP
70795714n3s	9	28	the	the	DET
70795714n3s	9	29	electrostatic	electrostatic	ADJ
70795714n3s	9	30	interactions	interaction	NOUN
70795714n3s	9	31	between	between	ADP
70795714n3s	9	32	adsorbates	adsorbate	NOUN
70795714n3s	9	33	and	and	CCONJ
70795714n3s	9	34	surfaces	surface	NOUN
70795714n3s	9	35	is	be	AUX
70795714n3s	9	36	often	often	ADV
70795714n3s	9	37	neglected	neglect	VERB
70795714n3s	9	38	in	in	ADP
70795714n3s	9	39	molecular	molecular	ADJ
70795714n3s	9	40	dynamics	dynamic	NOUN
70795714n3s	9	41	simulations	simulation	NOUN
70795714n3s	9	42	because	because	SCONJ
70795714n3s	9	43	of	of	ADP
70795714n3s	9	44	the	the	DET
70795714n3s	9	45	increased	increase	VERB
70795714n3s	9	46	computational	computational	ADJ
70795714n3s	9	47	cost	cost	NOUN
70795714n3s	9	48	and	and	CCONJ
70795714n3s	9	49	difficulty	difficulty	NOUN
70795714n3s	9	50	of	of	ADP
70795714n3s	9	51	implementation	implementation	NOUN
70795714n3s	9	52	.	.	PUNCT
70795714n3s	10	1	our	our	PRON
70795714n3s	10	2	new	new	ADJ
70795714n3s	10	3	mm	mm	PROPN
70795714n3s	10	4	-	-	PUNCT
70795714n3s	10	5	flucq	flucq	PROPN
70795714n3s	10	6	potential	potential	NOUN
70795714n3s	10	7	allows	allow	VERB
70795714n3s	10	8	us	we	PRON
70795714n3s	10	9	to	to	PART
70795714n3s	10	10	more	more	ADV
70795714n3s	10	11	properly	properly	ADV
70795714n3s	10	12	describe	describe	VERB
70795714n3s	10	13	a	a	DET
70795714n3s	10	14	metal	metal	NOUN
70795714n3s	10	15	surface	surface	NOUN
70795714n3s	10	16	's	's	PART
70795714n3s	10	17	response	response	NOUN
70795714n3s	10	18	to	to	ADP
70795714n3s	10	19	impinging	impinge	VERB
70795714n3s	10	20	charged	charge	VERB
70795714n3s	10	21	species	specie	NOUN
70795714n3s	10	22	in	in	ADP
70795714n3s	10	23	a	a	DET
70795714n3s	10	24	dynamic	dynamic	ADJ
70795714n3s	10	25	fashion	fashion	NOUN
70795714n3s	10	26	by	by	ADP
70795714n3s	10	27	allowing	allow	VERB
70795714n3s	10	28	the	the	DET
70795714n3s	10	29	charges	charge	NOUN
70795714n3s	10	30	on	on	ADP
70795714n3s	10	31	each	each	DET
70795714n3s	10	32	atomic	atomic	ADJ
70795714n3s	10	33	site	site	NOUN
70795714n3s	10	34	to	to	PART
70795714n3s	10	35	fluctuate	fluctuate	VERB
70795714n3s	10	36	in	in	ADP
70795714n3s	10	37	response	response	NOUN
70795714n3s	10	38	to	to	ADP
70795714n3s	10	39	the	the	DET
70795714n3s	10	40	local	local	ADJ
70795714n3s	10	41	electronic	electronic	ADJ
70795714n3s	10	42	environment	environment	NOUN
70795714n3s	10	43	.	.	PUNCT