-- S:- 1 i . , - I OFI ORNL P 2377 o 1 i • P 3. . • . on og se i .. SO 1156 |2.2 163 . 2.0 4 1.25 || 14 İLE u . : MICROCOPY RESOLUTION TEST CHART NATIONAL BUREAU OF STANDARDS - 1963 . SM/76-12 SLP 2 2 1966 CFSTI PRICES377 so it MN 60807-3 HC. & 1.07 - LEGAL NOTICE This report was prepared as an account of Governmont sponsored work, Nettaer the United States, nor the Commission, nor any person acting on bebail of the Commission: A. Alakes any warranty or representation, expressed or implied, with respect to the accu- racy, completeness, or usefulness of the information conlained in this report, or that the use of any information, apparatus, method, or process disclosed in this report may not infringe privately owned rights; or B. Absumes any llabilities with respect to the use of, or for damages reswung from the use of any information, apparatus, method, or process disclosed in this report. As used in the above, "person acting on behalf of the Commission" includes any om- ployce or contractor of the Commission, or employee of such contractor, to the oxtont that Buch employee or contractor of the Commission, or employoe of such contractor preparos, disseminates, or provides access lo, any information pursuant to his employment or contract with the Cummission, or his employment with such contractor. RELEASED FOZ ANNOUNCEMENT IN NUCLEAP. SCIENCE ABSTRACTS MULTILABORATORY INTERCOMPARISONS OF NEUTRON DOSIMETRY SYSTEMS* J. A. Auxier Health Physics Division, Oak Ridge National Laboratory Oak Ridge, Tennessee During the past ten years, several plants and laboratories in the United States have adopted and installed nuclear accident dosimetry systems. Because of the economic factor, the lack of adequate test facilities, or, in some cases, the pressure of time limitations resulting from the rash of accidents in 1958, most of these systems received only cursory testing and evaluation prior to their acceptance. However, health physicists now have more extensive radiation facilities at their disposal, particularly at the Oak Ridge National Laboratory, and more comprehensive and comparative studies of the accuracy and utility of the various systems have been initiated. In March of 1965, the first joint multilaboratory study was conducted at the ORNL DOSAR Facility with seven laboratories and production plants participating. Two exposures were made during which the Health Physics Research Reactor (HPRR) [1] was used in the burst mode to simulate acciden- tal nuclear excursions. On the first day, the HPRR was pulsed in a "low scatter" geometry with the dosimeter systems set up along an arc of 3 m radius. On the second day, the experiment was repeated with a 20-cm-thick *Research sponsored by the U. S. Atomic Energy Commission under contract with the Union Carbide Corporation. graphite moderator between the reactor and the dosimeters. During the first exposure, a live burro was also positioned along the arc to serve as a "phantom" complete with a heterngeneous and circulating source of blood were used for this purpose. The participants met two days after the second exposure to tabulate and compare results. After returning to their home installations and after further analysis of their data, they submitted revised estimates of the dose. In the fall of 1965, a second study was made primarily with the same participants. This was intended to test relative reproducibility with time as well as any modification which had appeared desirable and feasible. Future studies will include other installations and dosimeter systems and other radiation sources as well. (e.g., a small accelerator). Figure 1 shows the arrangement of the apparatus around the reactor for the first exposure, and Table I shows the results of the first two exposures. Rather than name the participating installations, they are designated here by a letter only, except for the DOSAR Facility. A more meaningful description is given in columns 2 and 3 of Table I, however, by listing the primary dosimeter components for neutrons and gamma rays, respectively. As most of the systems were calibrated for a fission spec- trum of neutrons, good agreement might be expected. The initial and revised estimates for the neutron and gamma-ray exposures are given in the last two columns. The results of the second exposure (i.e., with the graphite moderator in place) are shown also in Table I. In this case, there is an apparent increase in the variance of the reported results. Table II shows the ranges and averages for the data; the range cf results for total fluence and for two specific detectors is shown also. The results for the first two sets of experiments are esse:tially identical. The measurements made by the DOSAR Facility staff and repcaced in the table were made with threshold detector units [2,3] and photoluminescent dosimeters. [4,5] However, these systems were cross calibrated with other DOSAR standard instruments, including proportional counters, spectroneters, etc., so that the neutron and gamma-ray values should be accurate to within +5% and 18%, respectively, for one standard deviation. From these data and other auxiliary tests performed during the past few years, several conclusions may be drawn. The systems based on modera- tors with imbedded thermal detectors yield too high response in the low energy range from a few eV to 300 keV. The enhancement is of the order of 3 to 5. luclear emulsions and diode detectors (passive type) generally read low in this region; the emulsions show no neutron tracks for energies greater than thermal and less than about 0.5 MeV, and the response of the diodes decreases sharply below 250 to 300 keV. It seems reasonable that installations using the thermal neutron detectors in moderators might add either emulsions or diode detectors. If, in case of an accident, the two detectors give significantly different responses, the first higher than than a fission spectrum and that the two responses represent the extremes of the dose range. An average in this case would be better than either, and approximate limits of error would be established directly. Recent developments in the use of heavy particle track detection in solids with fission foil radiators permit extensive simplification and broader application of threshold detectors; [6] this may result in more widespread use of this versatile dosimeter system. Figure 2 shows a detector unit with glass plates for track detectors. Fission fragment tracks in glass rendered visible with a magnification of 100 by etching in hydrofluoric acid are shown in Fig. 3. REFERENCES . [41 [1] AUXIER, J. A. ,. Ilealth Phys. 11 (1965) 89. [?] HURST, G. S. et al., Rev. Sci. Instr. 27 3 (1956) 153. (3] REINHARDT, P. W., DAVIS, F. J., Health Phys. 1 (1958) 169. BERSARD, C. H. et al., Health Phys. 4 (1961) 236. [5] CHEKA, J. S., Health Phys. 10 (1964) 303. [6] KERR, 'G. D., STRICKLER, T. D., The application of solid-state nuclear track detectors to the Hurst threshold detector system, to be pub- lished in Health Physics. CAPTIONS Fig. 1. General view of the apparatus used in the first intercomparison experiment arranged for exposure to the HPRR. Fig. 2. Exploded view of the fission foil holder, foils, and glass detec- tors for the modified threshold detector system. Fig. 3. Photomicrograph of pits in glass caused by fission fragment bon- bardment and subsequent etching in hydrofluoric acid. Mo 1 R ' in a non line 2 . svetovnem *. ' STADI. W . RZEIT Bauen . ti, - . . . - - . - - - . :4 23 : SARE. - . Fig. 1 General view of the apparatus used in the first intercomparison experiment arranged for exposure to the HPRR و م . |+ " . م . م اما ما . ها و سه هزار و ا م . . . . ا حامیان ۲۰ 1 . همه ا " . ز ۹۰۰۰ . . والا ج : 1 وه TT T - وه اما ! س لم * . رس , ده مام ه . ها سه تار و - و .م . . . . . . . . . . . د ۱۰۰ . ۳ . 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R ول . : 1 : ا و او اف . و هوا م : . . سر I 1:11:: I و . واحد هی دوو • و " دو دید و دید . سي - ناهد م : - |- * ما = .ش ده است که نتمننننننننننننمه . . و . ق صص ستة من بمان باد و ها : : " و . . د !است و و قاد ا و م ا : ا او وح و لحد ما او . 4 * * * - ا " د بهم و 1 . 4 = وما و .. . .. .. . . . تم سے ره . . . .. . مه مه . . . . . .. . . .. . مهم و محدود و خه نن , او د با ما . ه وما ا و بارو . . : / ا . ..ان - د او ا ا ا م * 1 ما ا من ما مه له... . ۱۰ " | | | و مدام منظفة الانعت ۱۰تنه ننهه انا م. ۰ ند ندا ادب 11 م | 1 : : و .. سمممه : و ا ا ر ا 1 ا را به با و ا " ولد ا و م ا ر * . الا ا | ، * ؟ | " .، او * و | " و و ! و اپ 1 - . 4, : همه با = اذ Fig. 2 Expioded view of the fission foil holder, foils, and glass detectors for the modified threshold detector system | و . 1- ."بو و ، جک، ۰ و و " مي ۔ م . . . . ' وام که ها : - - - و به هاو . . ا : ' 11 F1 " , م 11 تم بهم ا - ة : م وه : . ه ه 24 ا ا ه هه ما . . : المدد به اد همه . . . ه . م. م " ا 1 - ...عمه.است . نل 140':: ...he is watro mister 3 . . . ! و المما ا ه ه : .ن.۱۹ . 4 : : .....::ما نه. ... . .. . . حابه و . ... :::::: وم = و ا : |: له . . . ادم و لہ مي OAK RIDGE NATIONAL LABORATORY |||||||||||||\'\'\'\'\' ** ' وہ انس . مع و - :وجه . ا م 11 داده و ه : . . . . : و ء هم - د ا رو * * مهم جدا : " . . ... " : - ،، به وه . - : ملا ... : 1 : و : : : 1 . بنا • ،، . :::: • • ۱۰:! - :: " . .: : و ما - و : و و م - . ا : :: 1 و - . مو، مر وجهه ع اد ء م : .•* . ! د . . : ء : : " : . م ع ا 1 :: : ا : ء م : ا م : ام بهوووو م . و و و و : نام : : نامیده . ها هم ه , المواره وه وهواء ما . . م : و. ه م . . 4 * * اه هه مه جدا و . بها * 14 د سم ها . " " " و کا مه ه * ب هم ا يه عي ءء * Fig. 3 Photomicrograph of pits in glass caused by fission fragment bombardment and subsequent etching in hydrofluoric acid 1000 , Table 1 RELATIVE DOSE VALUES OBTAINED BY THE VARIOUS INVESTIGATORS DURING THE FIRST INTERCOMPARISON STUDY Chief detector, neutron Burst B7!D, March 23, 1965 Fast Therma! Gamma neutrons neutrons rays (rads) (rads) (r) Chief detector, gamma Study group Burst B72D, March 24, 1965 Fast Thermal Gamma neutrons neutrons rays (rads) (rads) (r) A 0.6 73 0.5 32 Foils in moderator TLD and film - 462 3378 193 188 33 129a 30a -- - - - . ܫܝ - . - - - - - - - - - - B. 0.16 79 0.15 44 Foils on phantom Glass and film 468 337 132 120 - - - - - - - - - - - - -- DOSAR TDU Glass 58 81 0.30 22 320 300 3208 0.29a D TDU 56 79 24 Glass and film 332 356 0.19a S2 0.152 22a 21a 22a E 52 23 Modified TDU Glass and film 466 431 120 91 339a 333a 80 a 73a F Silicon diode 330 75 800 TDU 346 3162 0.20 Glass and film 52 Did not participate · "Revised two weeks after experiment. - * - --.. Table II RANGES AND AVERAGES OF DOSES AND FLUENCES REPORTED BY THE VARIOUS INVESTIGATORS DURING THE FIRST INTERCOMPARISON STUDY March 23 March 24 Range Fast neutrons Gammas 300 to 468 rads 52 to 79 r 75 to 193 rads 22 to 44 r. - Revised range - - - t -- Fast neutrons Gammas -- 316 to 339 rads 52 to 79 r 79 to 129 rads 22 to 44 r -- - *.. Average . Fast neutrons Gammas 384 rads 62 r 111 rads 29 r Revised average Fast neutrons Gammas 348 rads 60 r 96 rads 28 r Neutron fluence (total) Range Revised range (12.6 to 19) 1010 (12.6 to 19) 1010 (3.8 to 9)1010 (3.8 to 7.8)1010 In + Cd Range (0.02 to 0.47)1010 (0.02 to 0.48)1010 Cu Range 4.7 x 1010a (4.0 to 4.4)1010 Two identical values. . 1 - - - . .. - END - . - - - - - - C 1 ... ..1 DATE FILMED 10/24 / 66 ' . . 4 .